This link on MSDN is worth a visit: How to: Implement CopyToDataTable<T> Where the Generic Type T Is Not a DataRow
This adds an extension method that lets you do this:
// Create a sequence.
Item[] items = new Item[]
{ new Book{Id = 1, Price = 13.50, Genre = "Comedy", Author = "Gustavo Achong"},
new Book{Id = 2, Price = 8.50, Genre = "Drama", Author = "Jessie Zeng"},
new Movie{Id = 1, Price = 22.99, Genre = "Comedy", Director = "Marissa Barnes"},
new Movie{Id = 1, Price = 13.40, Genre = "Action", Director = "Emmanuel Fernandez"}};
// Query for items with price greater than 9.99.
var query = from i in items
where i.Price > 9.99
orderby i.Price
select i;
// Load the query results into new DataTable.
DataTable table = query.CopyToDataTable();