[c#] Best implementation for Key Value Pair Data Structure?

I think what you might be after (as a literal implementation of your question), is:

public class TokenTree
{
    public TokenTree()
    {
        tree = new Dictionary<string, IDictionary<string,string>>();
    }

    IDictionary<string, IDictionary<string, string>> tree; 
}

You did actually say a "list" of key-values in your question, so you might want to swap the inner IDictionary with a:

IList<KeyValuePair<string, string>>

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