[.net] WCF error: The caller was not authenticated by the service

set anonymous access in your virtual directory

write following credentials to your service

ADTService.ServiceClient adtService = new ADTService.ServiceClient();
adtService.ClientCredentials.Windows.ClientCredential.UserName="windowsuseraccountname";
adtService.ClientCredentials.Windows.ClientCredential.Password="windowsuseraccountpassword";
adtService.ClientCredentials.Windows.ClientCredential.Domain="windowspcname";

after that you call your webservice methods.

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