Using the angular.module API with an array at the end will tell angular to create a new module:
myApp.js
// It is like saying "create a new module"
angular.module('myApp.controllers', []); // Notice the empty array at the end here
Using it without the array is actually a getter function. So to seperate your controllers, you can do:
Ctrl1.js
// It is just like saying "get this module and create a controller"
angular.module('myApp.controllers').controller('Ctrlr1', ['$scope', '$http', function($scope, $http) {}]);
Ctrl2.js
angular.module('myApp.controllers').controller('Ctrlr2', ['$scope', '$http', function($scope, $http) {}]);
During your javascript imports, just make sure myApp.js is after AngularJS but before any controllers / services / etc...otherwise angular won't be able to initialize your controllers.